Karandras is my favorite, by a longshot. He's a combat machine and his fluff is just cool. And I'm a big fan of sneaky operatives. It's not easy to take the place of a previous pheonix lord, or so I'd heard. =)
In game, I'd go with Jain Zar though. I used her the other day and she DESTROYED 23 marines in close combat, ten of them being a beefed out veteran assault squad. She only missed 2 times in 4 turns of on and off assault(multiplayer turns), which is just rediculous on die rolling odds.
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